Patent · US Active

Pre-lithiated polyphenylene sulfide, polyphenylene sulfide-based solid electrolyte membrane, battery electrode sheet, quasi-solid-state lithium ion battery and method for manufacturing same

US11289737B2 · kind B2 · utility

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Key dates

Filing dateNov 20, 2020
Grant dateMar 29, 2022
Priority date
Expiry dateNov 20, 2040

Classification

  • Technology area (CPC Y)Emerging Cross-Sectional Technologies
  • CPC primaryY02P70/50
  • WIPO fieldMacromolecular chemistry, polymers
  • WIPO sectorChemistry

Abstract

A method for manufacturing a pre-lithiated polyphenylene sulfide with a high solid solubility of lithium includes; placing NMP, Li2S, and LiOH into a high-pressure reactor to obtain a mixture, and heating the mixture to 150-250° C. for a high-temperature dehydration for 2-5 h, and then cooling the mixture to 100° C. and adding p-DCB to the mixture for a reaction at 150-250° C. for 80-200 min; dropwise adding hydrochloric acid in an identical amount as that of the LiOH neutralize LiOH, and removing NMP and H2O by evaporation or sublimation, to obtain a dry mixed powder; and to the dry mixed powder, adding a chloride ion complexing agent to obtain a mixture, stirring the mixture to homogeneity, and placing the mixture in a sealed reactor for a reaction at 150-250° C. for 80-200 min, followed by washing and drying, to obtain the pre-lithiated polyphenylene sulfide.

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