Patent · US Expired

Layered manganese compound of the formula CA.sub.2 MN.sub.3 O.sub.8

US4049790A · kind A · utility

8Cited by
1References
2Claims
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Assignee

Inventors

Key dates

Filing dateJun 3, 1976
Grant dateSep 20, 1977
Priority date
Expiry dateJun 3, 1996

Classification

  • Technology area (CPC Y)Emerging Cross-Sectional Technologies
  • CPC primaryY02E60/10
  • WIPO fieldMaterials, metallurgy
  • WIPO sectorChemistry

Abstract

A new low temperature layered manganese compound of the formula Ca.sub.2 Mn.sub.3 O.sub.8 has unexpectedly been synthesized in pure form. The unit cell dimensions of this new compound have been determined by X-ray diffraction and reveal that the compound is monoclinic with lattice parameters of a=11.02 A, b=5.85 A, c=4.94 A, .alpha.=90.degree., .beta.=109.80.degree., .gamma.=90.degree.. The structure consists of pseudohexagonal Mn.sup.4+ sheets with similar oxygen sheets on either side, giving a distorted octahedral coordination to the Mn.sup.4+. Every fourth Mn.sup.4+ is missing in these layers, so their composition is Mn.sub.3 O.sub.8 with chains of coordination octahedra linked by common edges (rutile type arrangement). The Ca ions are situated between the Mn.sub.3 O.sub.8 layers. This new Ca.sub.2 Mn.sub.3 O.sub.8 compound is prepared in pure form by means of the solid solution precursor technique whereby solid solution, mixed metal carbonates of the desired metals (Ca and Mn) having the calcite structure are precipitated from mixtures of the solutions of the salts of calcium and manganese, said salts being selected from the group consisting of carbonates, nitrates, sulfates, o…

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