Patent · US Expired

Vinyl polybutadiene bisimide copolymers

US4216297A · kind A · utility

8Cited by
4References
9Claims
0Family size

Assignee

Inventors

Key dates

Filing dateFeb 13, 1978
Grant dateAug 5, 1980
Priority date
Expiry dateFeb 13, 1998

Classification

  • Technology area (CPC C)Chemistry; Metallurgy
  • CPC primaryC08K5/3415
  • WIPO fieldMacromolecular chemistry, polymers
  • WIPO sectorChemistry

Abstract

Vinyl polybutadiene bisimide copolymers which are peroxide curable are provided by two methods of formation. In the first method a bisimide cross-linked vinyl polybutadiene prepolymer is formed by combining a high vinyl content polybutadiene providing pendant vinyl groups with a bisimide in the presence of a first free radical initiating catalyst. The resultant cross-linked prepolymer is cured to a hard resin by the formation of additional cross-linkages through the pendant vinyl groups by heating the prepolymer to a temperature of at least about 300.degree. F. in the presence of a second free radical initiating catalyst. The second method discloses a method wherein the bisimide cross-linkages are formed in situ. In the second method, a high vinyl content polybutadiene providing pendant vinyl groups is reacted with maleic anhydride to form a maleic anhydride vinyl polybutadiene adduct. The adduct is subsequently combined with an aromatic polyamine and a free radical initiating catalyst. The mixture is heated to about 250.degree. F. to form a prepolymer having bisimide cross-linkages between the vinyl polybutadiene backbone segments. By continuing to heat the prepolymer to at least …

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.