Patent · US Expired

Continuous process for the preparation of nonrandom ethylene/acid copolymer

US4252924A · kind A · utility

29Cited by
7References
13Claims
0Family size

Assignee

Inventor

Key dates

Filing dateApr 5, 1979
Grant dateFeb 24, 1981
Priority date
Expiry dateApr 5, 1999

Classification

  • Technology area (CPC C)Chemistry; Metallurgy
  • CPC primaryC08F210/02
  • WIPO fieldMacromolecular chemistry, polymers
  • WIPO sectorChemistry

Abstract

There is provided a continuous, steady state process for the preparation of nonrandom ethylene/.alpha.,.beta.-ethylenically unsaturated carboxylic acid copolymers in at least 2 constant environment, stirred autoclaves in series wherein the first autoclave is maintained at the pressure in the range of 800 to 3000 atmospheres (11.8 to 44.1 kpsi) and at a temperature in the range of 120.degree. to 200.degree. C. in a single phase reaction mixture at the given concentration of copolymer in the reaction mixture and at the given acid comonomer content of the copolymer and wherein each succeeding autoclave is maintained at a temperature of at least 30.degree. C. in excess of the preceding autoclave. The compolymers thus obtained have a ratio of percent adjacent acid to weight percent acid in the copolymer of from above 0.44 to about 1.0. These copolymers have improved stiffness and are particularly useful in sheeting, blow molding, and packaging applications and for conversion to ionomers which are also useful for similar applications.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.