Patent · US Expired

Process for recovering triarylphosphine from poisoned rhodium catalyst systems

US4503255A · kind A · utility

1Cited by
8References
9Claims
0Family size

Assignee

Inventors

Key dates

Filing dateApr 29, 1982
Grant dateMar 5, 1985
Priority date
Expiry dateApr 29, 2002

Classification

  • Technology area (CPC Y)Emerging Cross-Sectional Technologies
  • CPC primaryY02P20/584
  • WIPO fieldOrganic fine chemistry
  • WIPO sectorChemistry

Abstract

A process for recovering re-usable triarylphosphine (e.g. triphenylphosphine) from rhodium catalyst residues poisoned by the presence of alkyldiarylphosphine (e.g. n-propyldiphenylphosphine) such as are obtained as spent catalyst residues from the hydroformylation of olefins. The process comprises subjecting the poisoned residues to evaporative separation under reduced pressure to separate a vapor comprising triarylphosphine from the rhodium and then mixing the condensed vapor with polar solvent and obtaining the triarylphosphine as a crystalline precipitate from the solvent. The crystalline phosphine is sufficiently free of poisons to be re-usable as a catalyst component in a hydroformylation process.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.