Patent · US Expired

Process for dimerizing lower .alpha.-olefins

US4709112A · kind A · utility

12Cited by
2References
5Claims
0Family size

Assignee

Inventors

Key dates

Filing dateDec 30, 1986
Grant dateNov 24, 1987
Priority date
Expiry dateDec 30, 2006

Classification

  • Technology area (CPC C)Chemistry; Metallurgy
  • CPC primaryC07C2531/24
  • WIPO fieldChemical engineering
  • WIPO sectorChemistry

Abstract

An improved process for dimerizing lower .alpha.-olefins using a novel nickel-containing Ziegler catalyst system including PA1 (A) an organic acid salt or complex of nickel, PA1 (B) a trialkylaluminum, PA1 (C) a trivalent phosphorus compound of the formula: EQU PR.sup.1 R.sup.2 R.sup.3 (I) EQU P(NR.sup.1.sub.2).sub.3 (II) EQU P(OR.sup.1).sub.3 (III) PA1 wherein R.sup.1, R.sup.2, R.sup.3 are alkyl, cycloalkyl, aryl or aralkyl, PA1 (D) a fluorinated isopropanol of the formula: ##STR1## wherein m and n are in 4.ltoreq.m+n.ltoreq.6, and optionally (E) a catalyst co-activator: halogenated compounds of the formulae: ##STR2## wherein X is halogen, R.sup.4, R.sup.5, R.sup.6 are alkyl, and n is 1 to 3, and further optionally, PA1 (F) a compound selected from aliphatic alcohol and aliphatic carboxylic acid or ester thereof, which yields the dimers with high selectivity of isomers and uniformity of the catalyst without corrosion of the apparatus.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.