Patent · US Expired

Phosphonite-and phosphinite-promoted ruthenium - cobalt catalysts for the dealkoxyhydroxymethylation of acetals to form glycol ethers

US4895818A · kind A · utility

14Cited by
12References
6Claims
0Family size

Assignee

Inventors

Key dates

Filing dateAug 31, 1988
Grant dateJan 23, 1990
Priority date
Expiry dateAug 31, 2008

Classification

  • Technology area (CPC B)Performing Operations; Transporting
  • CPC primaryB01J2531/845
  • WIPO fieldChemical engineering
  • WIPO sectorChemistry

Abstract

Ruthenium cobalt- or cobalt-containing catalysts which have been promoted with phosphonites or phosphinites effectively catalyze the dealkoxyhydroxymethylation of aldehyde acetals to form glycol monoethers. Methylal, for example, may be reacted with syngas, i.e., CO and H.sub.2, in the presence of these phosphonite- or phosphinite-promoted cobalt or ruthenium- cobalt catalysts to form the monomethyl ether of ethylene glycol. In a like manner acetaldehyde may be converted to the corresponding propylene glycol monoether. The process may advantageously be carried out with high yields and selectivities in the presence of a polar or non-polar organic solvent in combination with the catalyst system of this invention. The invention is also directed to the phosphonite- or phosphinite-promoted cobalt and ruthenium-cobalt catalyst systems per se.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.