Patent · US Expired

Process of linking nucleosides with a siloxane bridge

US5214134A · kind A · utility

488Cited by
1References
24Claims
0Family size

Assignee

Inventors

Key dates

Filing dateSep 12, 1990
Grant dateMay 25, 1993
Priority date
Expiry dateSep 12, 2010

Classification

  • Technology area (CPC C)Chemistry; Metallurgy
  • CPC primaryC07H23/00
  • WIPO fieldOrganic fine chemistry
  • WIPO sectorChemistry

Abstract

A method of linking nucleosides with a siloxane bridge comprising reacting a 3'-silylated-5'-protected nucleoside with an unprotected nucleoside is disclosed. The silylated and unprotected nucleosides may be either monomeric nucleosides or the terminal nucleosides of an oligonucleotide or oligonucleotide analog. A method of synthesizing an oligonucleotide analog having siloxane internucleoside linkages is also disclosed. The method of synthesis comprises silylating a 5'-protected nucleoside with a bifunctional silylating reagent to form a 3'-silylated nucleoside, reacting the silylated nucleoside with an unprotected nucleoside in the presence of a base catalyst and repeating these steps to form an oligonucleotide analog. A modified solid phase synthesis method for preparing an oligonucleotide analog having siloxane internucleoside linkages is also disclosed.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.