Patent · US Expired

Continuous preparation of low unsaturation polyoxyalkylene polyether polyols with continuous additon of starter

US5689012A · kind A · utility

65Cited by
14References
31Claims
0Family size

Assignee

Inventors

Key dates

Filing dateJul 18, 1996
Grant dateNov 18, 1997
Priority date
Expiry dateJul 18, 2016

Classification

  • Technology area (CPC C)Chemistry; Metallurgy
  • CPC primaryC08G65/2696
  • WIPO fieldMacromolecular chemistry, polymers
  • WIPO sectorChemistry

Abstract

A continuous process for the preparation of polyoxyalkylene polyethers using DMC catalysts as the polyoxyalkylation catalyst employs continuous addition of alkylene oxide in conjunction with continuous addition of starter and catalyst to a continuous oxyalkylation reactor. Despite the continuous introduction of starter, the molecular weight distribution of the polyether product is quite narrow, as indicated by the exceptionally low polydispersity of the product. The presence of low molecular weight species during the majority of the polyoxyalkylation also substantially eliminates extremely high molecular weight fractions having molecular weights greater than 100,000 Da, again without appreciably broadening molecular weight distribution. By withdrawing intermediate molecular weight polyether product or diverting a portion of the end product to prepare a catalyst/starter mixture, rapid and sustained reaction rates can be achieved while employing low molecular weight starters. Continuous build ratios in excess of 0.98 can be achieved.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.