Patent · US Expired

Process for the preparation of E-caprolactam

US5717089A · kind A · utility

8Cited by
11References
15Claims
0Family size

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Inventors

Key dates

Filing dateMar 15, 1996
Grant dateFeb 10, 1998
Priority date
Expiry dateMar 15, 2016

Classification

  • Technology area (CPC C)Chemistry; Metallurgy
  • CPC primaryC07D201/08
  • WIPO fieldOrganic fine chemistry
  • WIPO sectorChemistry

Abstract

Process for the preparation of .epsilon.-caprolactam starting from an aldehyde compound comprising at least one member from among 5-formylvaleric acid, ester or amide in which the aldehyde compound is allowed to react in the presence of ammonia and hydrogen and a subsequent cyclization of the reaction products thus formed (.epsilon.-caprolactam-precursors) to .epsilon.-caprolactam is performed in the presence of water, involved the combination of steps PA1 (a) contacting the 5-formylvaleric acid, ester or amide with ammonia and water under non-hydrogenation conditions, PA1 (b) contacting the resulting mixture of step (a) with hydrogen in the presence of ammonia under hydrogenation conditions, wherein the water content is greater than 10 wt. %, PA1 (c) heating the resulting mixture of step (b) at a temperature between 200.degree. and 350.degree. C. in order to convert the reaction products of step (b) to .epsilon.-caprolactam.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.