Patent · US Expired

Process for preparing alkanediols

US5731478A · kind A · utility

15Cited by
9References
19Claims
0Family size

Assignee

Inventors

Key dates

Filing dateOct 15, 1996
Grant dateMar 24, 1998
Priority date
Expiry dateOct 15, 2016

Classification

  • Technology area (CPC C)Chemistry; Metallurgy
  • CPC primaryC07C45/58
  • WIPO fieldOrganic fine chemistry
  • WIPO sectorChemistry

Abstract

An alkanediol such as 1,3-propanediol is prepared in a process which involves reacting an alkylene oxide with carbon monoxide and hydrogen in an essentially non-water-miscible solvent in the presence of a non-phosphine-ligated cobalt or rhodium catalyst and a manganese porphyrine promoter to produce an intermediate product mixture containing a hydroxyalkanal in an amount less than 15 wt %; extracting the hydroxyalkanal from the intermediate product mixture into an aqueous liquid at a temperature less than about 100.degree. C. and separating the aqueous phase containing hydroxyalkanal from the organic phase containing cobalt catalyst; hydrogenating the hydroxyalkanal in the aqueous phase to an alkanediol; and recovering the alkanediol. The process enables the production of an alkanediol such as 1,3-propanediol in high yields and selectivity without the use of a phosphine ligand with the cobalt or rhodium catalyst.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.