Patent · US Expired

Method of hydrogenation of living polymer

US6020439A · kind A · utility

17Cited by
12References
7Claims
0Family size

Assignee

Inventors

Key dates

Filing dateJan 26, 1998
Grant dateFeb 1, 2000
Priority date
Expiry dateJan 26, 2018

Classification

  • Technology area (CPC B)Performing Operations; Transporting
  • CPC primaryB01J2531/46
  • WIPO fieldMacromolecular chemistry, polymers
  • WIPO sectorChemistry

Abstract

A method for hydrogenating living polymers that include mainly conjugated double bond monomers and aromatic vinyl monomers. At least one conjugated diene compound is polymerized or copolymerized in an inert solvent by using a polymerization initiator of organic alkali metal. The produced polymer is contacted with hydrogen in the presence of a catalyst. The catalyst is formed of a cyclopentadienyl titanium compound represented by: ##STR1## wherein R.sub.1, R.sub.2 and R.sub.3 are independently selected from halogen groups, C.sub.1 -C.sub.8 alkyl groups, C.sub.1 -C.sub.8 alkoxy groups, C.sub.6 -C.sub.20 aryloxy groups, C.sub.6 -C.sub.20 cycloalkyl groups, silyl groups, and carbonyl groups. A cocatalyst is provided of alkoxylithium compound represented by: EQU R.sub.4 O--Li wherein R.sub.4 is a hydrocarbon. This cocatalyst selectively hydrogenates the unsaturated double bonds in the conjugated diene units of the living polymer.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.