Patent · US Expired

Process for the manufacture of halocarbons and selected compounds and azeotropes with HF

US6291730A · kind A · utility

17Cited by
20References
12Claims
0Family size

Assignee

Inventors

Key dates

Filing dateJan 28, 1998
Grant dateSep 18, 2001
Priority date
Expiry dateJan 28, 2018

Classification

  • Technology area (CPC Y)Emerging Cross-Sectional Technologies
  • CPC primaryY02P20/582
  • WIPO fieldOrganic fine chemistry
  • WIPO sectorChemistry

Abstract

A liquid phase process is disclosed for producing halogenated alkane adducts of the formula: CAR.sup.1 R.sup.2 CBR.sup.3 R.sup.4 (where A, B, R.sup.1, R.sup.2, R.sup.3, and R.sup.4 are as defined in the specification) which involves contacting a corresponding halogenated alkane, AB, with a corresponding olefin, CR.sup.1 R.sub.2.dbd.C.sup.3 R.sup.4 in a dinitrile or cyclic carbonate ester solvent which divides the reaction mixture into two liquid phases and in the presence of a catalyst system containing: (i) at least one catalyst selected from monovalent and divalent copper; and optionally (ii) a promoter selected from aromatic or aliphatic heterocyclic compounds which contain at least one carbon-nitrogen double bond in the heterocyclic ring. When hydrochlorofluorocarbons are formed, the chlorine content may be reduced by reacting the hydrochlorofluorocarbons with HF. New compounds disclosed include CF.sub.3 CF.sub.2 CCl.sub.2 CH.sub.2 CCl.sub.3, CF.sub.3 CCl.sub.2 CH.sub.2 CH.sub.2 Cl and CF.sub.3 CCl.sub.2 CH.sub.2 CHClF. These compounds are useful as intermediates for producing hydrofluorocarbons. Azeotropes of CClF.sub.2 CH.sub.2 CF.sub.3 with HF and azeotropes of CF.sub.3 CH.s…

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.