Patent · US Expired

Gel-free process for making functionalized anionically polymerized polymers

US6462143B1 · kind B1 · utility

5Cited by
10References
58Claims
0Family size

Assignee

Inventors

Key dates

Filing dateJan 20, 1999
Grant dateOct 8, 2002
Priority date
Expiry dateJan 20, 2019

Classification

  • Technology area (CPC C)Chemistry; Metallurgy
  • CPC primaryC08F8/42
  • WIPO fieldMacromolecular chemistry, polymers
  • WIPO sectorChemistry

Abstract

This invention relates to a gel-free process for making functionalized polymers. When multi-alkali metal initiators are used to make these polymers anionically, the process comprises anionically polymerizing at least one monomer with a multi-alkali metal initiator in a hydrocarbon solvent, capping the polymer by adding to the polymer a capping agent that reacts with the ends of the polymer chains such that strongly associating chain ends are formed wherein a strongly associating gel is formed, and, finally, adding a trialkyl aluminum compound to the gel. The important characteristic of the capping agent herein is that it will cap the living polymer and will add a functional group to the polymer chain end which will be strongly associating in the hydrocarbon solvent. In a second embodiment, the present invention relates to a process for making such polymers which comprises anionically polymerizing them as described and adding to the polymer a trialkyl aluminum compound before the alkali metal reacts with the capping agent-functionalized chain ends. Finally, the polymer is capped by adding the above-described capping agent. In the first embodiment, a gel is formed and then removed. I…

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.