Patent · US Expired

Synthesis for 4,10-dinitro-2,6,8,12-tetraoxa-4,10-diazatetracyclo[5.5.0.05,903,11]-dodecane

US6512113B1 · kind B1 · utility

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20Claims
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Inventors

Key dates

Filing dateJun 8, 2000
Grant dateJan 28, 2003
Priority date
Expiry dateJul 29, 2020

Classification

  • Technology area (CPC C)Chemistry; Metallurgy
  • CPC primaryC06B25/34
  • WIPO fieldOrganic fine chemistry
  • WIPO sectorChemistry

Abstract

A process for preparing 4,10-dinitro-2,6,8,12-tetraoxa-4,10-diazatetracyclo[5.5.0.05,903,11]-dodecane involves reacting at least one hexa-substituted piperazine derivative with at least one nitrate source and optionally at least one strong acid and heating the mixture to a temperature sufficient to induce an exothermic initial stage of the between the hexa-substituted piperazine derivative and the nitrate source. The mixture is maintained at a temperature in a range of at least ambient to not more than about 80° C. during the exothermic initial stage and at least a portion of a subsequent non-exothermic intermediate stage of the reaction by cooling the mixture during at least a portion of the exothermic initial stage of the reaction so that the reaction proceeds in a controlled manner. The mixture is then cooled to a temperature sufficiently low to prevent commencement of an exothermic NOx autocatalytic stage.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.