Patent · US Expired

Method for resolving racemic mixtures of 5-substituted 4-hydroxy-2-furanones

US6613919B2 · kind B2 · utility

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2References
15Claims
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Assignee

Inventor

Key dates

Filing dateJun 28, 2002
Grant dateSep 2, 2003
Priority date
Expiry dateJun 28, 2022

Classification

  • Technology area (CPC C)Chemistry; Metallurgy
  • CPC primaryC07D307/60
  • WIPO fieldOrganic fine chemistry
  • WIPO sectorChemistry

Abstract

This invention affords a solution to the technical problem of obtaining one or both enantiomers of 5-substituted 4-hydroxyfuran-2-ones in pure form by resolution with enantiomerically pure bases. Racemic mixtures of 5-substituted 4-hydroxy-2(5H)-furanones, including 5-substituted and 5,5-disubstituted, 4-hydroxy and 3,4-dihydroxy furanones are separated into pure enantiomers by crystallization with an enantiomerically pure base, such as cinchonidine. In specific solvent mixtures, for example, 95% ethanol, the diastereomerically pure salt of one enantiomer crystallizes. The enantiomerically pure furanone can then be obtained simply by filtration and treatment of the salt with an acid, for example, trifluoracetic acid, followed by precipitation with water, filtration and drying. Moreover, the other enantiomer may be equally obtained in pure form by evaporation of the mother liquor, followed by the same treatment of the salt as described before.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.