Patent · US Active

Method for determining isotopic clusters and monoisotopic masses of polypeptides on mass spectra of complex polypeptide mixtures and computer-readable medium thereof

US8321153B2 · kind B2 · utility

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17Claims
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Key dates

Filing dateDec 28, 2007
Grant dateNov 27, 2012
Priority date
Expiry dateMar 11, 2029

Classification

  • Technology area (CPC H)Electricity
  • CPC primaryH01J49/0036
  • WIPO fieldElectrical machinery, apparatus, energy
  • WIPO sectorElectrical engineering

Abstract

Disclosed herein is a method of finding an isotopic cluster in a polypeptide and determining the monoisotopic mass of the cluster. The method comprises an algorithm for finding an isotopic cluster based on a probabilistic model, defined by each of peaks in the isotopic cluster, and determining the monoisotopic mass of the isotopic cluster. The probabilistic model of the isotopic cluster includes characteristic functions for mass, that is, a function of the ratio of two peak intensities, and a function of the product of two ratios obtained from three peaks. These characteristic functions for mass define the shape of peaks acceptable in an actual isotopic cluster for the mass of any isotopic cluster. The algorithm of finding the isotopic cluster based on the functions uses the characteristics to score the degree of the approximation of any isotopic cluster to the spectral shape of a theoretical cluster.

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