Patent · US Expired

Method of making asymmetric de ring intermediates for the synthesis of camptothecin and camptothecin analogs

US5428166A · kind A · utility

3Cited by
7References
26Claims
0Family size

Assignee

Inventor

Key dates

Filing dateApr 12, 1994
Grant dateJun 27, 1995
Priority date
Expiry dateApr 12, 2014

Classification

  • Technology area (CPC C)Chemistry; Metallurgy
  • CPC primaryC07D491/04
  • WIPO fieldOrganic fine chemistry
  • WIPO sectorChemistry

Abstract

A method of making racemic DE ring intermediates for the synthesis of camptothecin and camptothecin analogs employing novel intermediates of Formula XX and XXI: ##STR1## as precursors to the DE ring intermediate. The present invention also provides camptothecin analog of Formula I-A ##STR2## wherein: Hal is a halogen is selected from the group consisting of F, Cl, and Br; PA1 R may be loweralkyl; PA1 R.sub.1 may be H, loweralkyl, loweralkoxy, or halo; PA1 R.sub.2, R.sub.3, R.sub.4, and R.sub.5 may each independently be H, amino, hydroxy, loweralkyl, loweralkoxy, loweralkyl-thio, di(loweralkyl)amino, cyano, methylenedioxy, formyl, nitro, halo, trifluoromethyl, amninomethyl, azido, amido, hydrazino, or any of the twenty standard amino acids bonded to the A ring via the amino-nitrogen atom. Additionally, novel compounds useful in the preparation of the compounds of Formula I-A are also provided.

Source: USPTO / EPO open patent data. Objective bibliographic and citation counts.